[Pollution Characteristics and Source Apportionment of Ambient PM2.5 During Four Seasons in Yantai City]
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Published on: June 20, 2016
Tong Liu1, Xiao-Jun Wang2, Qian Chen2
1State Environmental Protection Key Laboratory of Urban Ambient Air Particulate Matter Pollution Prevention and Control, College of Environmental Science and Engineering, Nankai University, Tianjin 300071, China.
Abstract:
PM2.5 samples were collected at three sites in Yantai City during all four seasons of 2016-2017, and the mass concentration and chemical composition characteristics were analyzed. The CMB model was used to calculate source apportionment of ambient PM2.5, and the backward trajectory cluster and PSCF were used to analyze the transport flow and potential source regions. The results showed that the average mass concentrations of PM2.5 in winter, spring, summer, and autumn in Yantai were (89.45±56.80), (76.78±28.44), (32.65±17.92) and (57.32±24.60) μg·m-3, respectively. The PM2.5 concentration showed a significant seasonal variation (P<0.01). The contribution of PM2.5 sources was as follows:secondary nitrate (20.3%) > crustal dust (15.7%) > vehicle exhaust (14.9%) > coal combustion (13.8%) > secondary sulphate (12.8%) > SOC (6.1%) > cement dust (5.5%) > sea salt source (2.9%). It can be seen that the predominant sources were secondary sources, crustal dust, vehicle exhaust, and coal combustion. The sources of nitrate in spring and of crustal dust were important contributors. The contribution of sulfate in summer was prominent, and the proportion of coal combustion was high in autumn and winter. Yantai City's airflow transport and potential source regions also showed significant seasonal changes:winters were mainly affected by short-distance transport in Yantai City; summers were mainly affected by the coastal of eastern Yantai City and local areas; springs and autumns were mainly affected by regional transmission in the northeast and in the eastern coastal areas of Shandong Province and by local sources in Yantai City.
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