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Nonequilibrium magnetic properties in oxygen-rich LaMnO3 nanoparticles
Kaiyuan Xue1, Feifei He1, Jiang Zhang1
1School of Physics and Optoelectronics, South China University of Technology, Guangzhou, People's Republic of China.
None:
Nonequilibrium magnetic properties of oxygen-rich LaMnO3.21 nanoparticles have been investigated by comprehensive magnetic measurements. The composition falls in the metamagnetic canted spin region of the magnetic phase diagram. However, the zero-field-cooling memory effect and frequency-dependent AC susceptibility reveal a re-entrant glassy state at low temperature. In contrast to the super-spin glass or cluster glass that re-enter from the high-temperature ferromagnetic state in previous studies, analyses based on the power law and Vogel-Fulcher law indicate strongly a conventional spin glass nature. As the magnetic field increases, an anomalous enhancement of the irreversible temperature is observed, suggesting a field-induced nonequilibrium magnetic state. These results can be understood by considering the interaction between the antiferromagnetic clusters and the metamagnetic canted-spin matrix inside the nanoparticles.
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