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Muhammad Waqas1,2,3, Shamshad Ali1,2, Chao Feng2

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This review explores advanced separators for high-temperature lithium-ion batteries (LIBs). It details recent progress in monolayer and multilayer separators to enhance thermal stability and battery performance.

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Area of Science:

  • Materials Science
  • Electrochemistry
  • Energy Storage

Background:

  • Lithium-ion batteries (LIBs) are vital for renewable energy integration and high-power applications due to their excellent energy density and longevity.
  • However, LIBs face significant challenges at high temperatures, primarily due to thermal instability within the battery.
  • The battery separator is a critical component influencing high-temperature performance and overall battery safety.

Purpose of the Study:

  • To review recent advancements in separator technologies for high-temperature LIBs.
  • To analyze the structural layered formation and preparation methodologies of these advanced separators.
  • To identify future challenges and research directions for high-temperature LIB separator development.

Main Methods:

  • Literature review of recent studies on separator technologies for high-temperature LIBs.
  • Analysis of structural characteristics, including monolayer and multilayer formations.
  • Discussion of preparation methodologies and their impact on separator properties.

Main Results:

  • High thermal stability, minimal shrinkage, and robust mechanical strength are essential for high-temperature LIB separators.
  • Advanced monolayer and multilayer separators show promise in addressing thermal stability issues.
  • Optimized porosity, ionic conductivity, and electrolyte uptake are crucial for efficient high-temperature operation.

Conclusions:

  • Separator technology is key to enabling sustainable and high-performance LIBs at elevated temperatures.
  • Recent progress in separator design and fabrication offers pathways to overcome current limitations.
  • Further research into novel materials and structures is needed to achieve remarkable performance in demanding high-temperature environments.