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Interface in Solid-State Lithium Battery: Challenges, Progress, and Outlook.

Syed Atif Pervez1, Musa Ali Cambaz1, Venkataraman Thangadurai2

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ACS Applied Materials & Interfaces
|May 31, 2019
PubMed
Summary

All-solid-state batteries (ASSBs) offer enhanced safety and performance but face challenges from high interfacial resistance. This study investigates interfacial behavior in oxide and sulfide solid electrolytes to improve charge transfer and battery efficiency.

Keywords:
Li dendritesinterface resistanceinterfacial characterizationsolid-electrolytesolid-state battery

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Area of Science:

  • Materials Science
  • Electrochemistry
  • Energy Storage

Background:

  • All-solid-state batteries (ASSBs) utilizing inorganic solid electrolytes offer significant advantages over conventional lithium-ion batteries, including improved safety, higher energy density, extended cycle life, and reduced costs.
  • Practical implementation of ASSBs is hindered by substantial resistance at the solid-solid electrode-electrolyte interfaces, impeding efficient charge transfer.
  • The precise mechanisms underlying this interfacial resistance are not fully elucidated, but involve complex chemical, electrochemical, and chemo-mechanical interactions.

Purpose of the Study:

  • To investigate the interfacial behavior of lithium and cathodes within oxide and sulfide inorganic solid electrolytes.
  • To understand how these interfacial characteristics influence overall battery performance.
  • To summarize current research on high resistance at anodic and cathodic interfaces and the scientific/engineering solutions.

Main Methods:

  • Analysis of interfacial phenomena in oxide and sulfide solid electrolytes.
  • Evaluation of charge transfer mechanisms at electrode-electrolyte interfaces.
  • Review of existing literature on interfacial resistance mitigation strategies.

Main Results:

  • Detailed examination of interfacial behavior in different solid electrolyte systems (oxide and sulfide).
  • Correlation established between interfacial characteristics and overall battery performance metrics.
  • Identification of key chemical, electrochemical, and chemo-mechanical factors contributing to interfacial resistance.

Conclusions:

  • Understanding and mitigating interfacial resistance is critical for advancing ASSB technology.
  • Specific interfacial behaviors in oxide and sulfide electrolytes significantly impact battery performance.
  • A comprehensive overview of solutions provides a roadmap for future ASSB development.