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Updated: Jan 22, 2026

Measurement of Ultrafast Vibrational Coherences in Polyatomic Radical Cations with Strong-Field Adiabatic Ionization
Published on: August 6, 2018
Vibrational Raman scattering from coherently excited molecular ions in a strong laser field
Abstract:
We report on a pump-probe investigation of vibrational Raman scattering from coherently excited N2+ ions. It is found that the Raman signals produced by the inelastic scattering of the probe pulse from molecular ions can be dramatically enhanced when the probe laser is resonant with electronic transitions in N2+ ions. The Raman signal can be amplified at 428 nm wavelength due to the presence of population inversion in N2+ ions.
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