Ferromagnetic resonance studies of strain tuned Bi:YIG films

Bismuth-doped Yttrium iron garnet (Bi:YIG) thin films known for large magneto-optical activity with low losses still need to get probed for its magnetization dynamics. We demonstrate a controlled tuning of magnetocrystalline anisotropy in Bi-doped Y₃Fe₅O₁₂ (Bi:YIG) films of high crystalline quality using growth induced epitaxial strain on [1 1 1]-oriented Gd₃Ga₅O₁₂ (GGG) substrate. We optimize a growth protocol to get thick highly-strained epitaxial films showing large magneto-crystalline anisotropy, compare to thin films prepared using a different protocol. Ferromagnetic resonance measurements establish a linear dependence of the out-of-plane uniaxial anisotropy on the strain induced rhombohedral distortion of Bi:YIG lattice. Interestingly, the enhancement in the magnetoelastic constant due to an optimum substitution of Bi³⁺ ions with strong spin orbit coupling does not strongly affect the precessional damping (∼[Formula: see text]). Large magneto-optical activity, reasonably low damping, large magnetocrystalline anisotropy and large magnetoelastic coupling in Bi:YIG are the properties that may help Bi:YIG emerge as a possible material for photo-magnonics and other spintronics applications.