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Plasmonic Core-Shell Silicon Carbide-Graphene Nanoparticles.

Devin Coleman1, Lorenzo Mangolini1

  • 1Material Science & Engineering Program and Mechanical Engineering Department, University of California, Riverside, Riverside, California 92521, United States.

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|August 29, 2019
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Summary

We synthesized silicon carbide nanoparticles with graphene coatings, confirming their infrared plasmonic behavior. Plasma process control tunes size and optical properties for diverse applications.

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Area of Science:

  • Materials Science
  • Nanotechnology
  • Plasma Physics

Background:

  • Silicon carbide (SiC) nanoparticles are investigated for unique electronic and optical properties.
  • Graphene coatings can enhance nanoparticle functionality and stability.
  • Plasmonic behavior in nanomaterials offers potential for advanced optical applications.

Purpose of the Study:

  • To synthesize silicon carbide nanoparticles with graphene shells.
  • To characterize the optical response and confirm plasmonic behavior.
  • To investigate the influence of synthesis parameters on nanoparticle properties.

Main Methods:

  • A multistep, low-temperature plasma process for in-flight nucleation, carbonization, and graphene coating.
  • Optical characterization, including surface plasmon resonance (SPR) measurements in the infrared region.
  • High-temperature optical characterization to assess property stability.

Main Results:

  • Successful synthesis of silicon carbide nanoparticles with monolayer to few-layer graphene coatings.
  • Observation of surface plasmon resonance in the infrared spectrum, confirming plasmonic behavior.
  • Demonstrated control over nanoparticle size and SPR peak position by tuning plasma parameters.
  • Excellent agreement between experimental data and a simplified dielectric permittivity model.
  • Confirmation of stable optical properties at elevated temperatures.

Conclusions:

  • The developed plasma process enables controlled synthesis of graphene-coated SiC nanoparticles.
  • These nanoparticles exhibit tunable infrared plasmonic properties.
  • The material's thermal stability makes it suitable for high-temperature applications.
  • Potential applications in areas requiring infrared plasmonics and stable nanomaterials.