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From aerospace to screen: Multifunctional poly(benzoxazine)s based on different triarylamines for electrochromic,
Yan Wang1, Haiying Niu2, Qingyi Lu1
1Key Laboratory of Functional Inorganic Material Chemistry, Ministry of Education, Department of Macromolecular Science and Engineering, School of Chemical, Chemical Engineering and Materials, Heilongjiang University, Harbin 150086, PR China.
Abstract:
Four kinds of main-chain benzoxazine polymers (PBZ) containing triarylamine (TAA) units were synthesized by Mannich reaction and characterized by 1H nuclear magnetic resonance (NMR), Fourier transform infrared (FT-IR) techniques, etc. Thermal, optical, photophysical and electrochemical properties were studied. The 50% of char residue is left in N2 at 800 °C. The polymers are soluble in common organic solvents and easily spin-coated onto indium‑tin oxide (ITO) coated glass substrates. All the polymers have voltage window ranging from 0 to 1.8 V, and the colors change from yellowish to dark red when voltage is applied. Meanwhile, device assembled from polymer exhibit significant color changes. Furthermore, the polymers also have promising potential application in explosive detection and resistance memory devices.
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