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RETRACTED: Nanostructured Nickel Nitride with Reduced Graphene Oxide Composite Bifunctional Electrocatalysts for an
Feng Wang1, Dongsheng Zhao1, Linbao Zhang2
1Department of Chemistry, College of Science, North University of China, Taiyuan 030051, China.
Abstract:
A three-dimensional nickel nitride with reduced graphene oxide composite on nickel foam (s-X, where s represents Ni3N/rGO@NF and the annealing temperature X can be 320, 350, or 380) electrode has been fabricated through a facile method. We demonstrate that s-350 has excellent urea oxidation reaction (UOR) activity, with a demanded potential of 1.342 V to reach 10 mA/cm2 and bears high hydrogen evolution reaction (HER) activity. It provides a low overpotential of 124 mV at 10 mA/cm2, which enables the successful construction of its two-electrode alkaline electrolyzer (s-350||s-350) for water-urea splitting. It merely requires a voltage of 1.518 V to obtain 100 mA/cm2 and is 0.145 V lower than that of pure water splitting. This noble metal-free bifunctional electrode is regarded as an inexpensive and effective water-urea electrolysis assisted hydrogen production technology, which is commercially viable.
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