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Facile Fabrication of Ce/V-Modified Multi-Channel TiO2 Nanotubes and Their Enhanced Selective Catalytic Reduction
Xiaosheng Huang1,2, Guodong Zhang1, Zhicheng Tang1,3
1State Key Laboratory for Oxo Synthesis and Selective Oxidation, National Engineering Research Center for Fine Petrochemical Intermediates, Lanzhou Institute of Chemical Physics, Chinese Academy of Sciences, Lanzhou, 730000, P. R. China.
Abstract:
To optimize one-dimensional (1D) TiO2 nanofibers, tailor-made multi-channel TiO2 nanotubes have been successfully fabricated by electrospinning technology. After loading with Ce and V, the CeVTi-tube catalyst exhibited a broad working temperature window and acceptable resistance to H2 O and SO2 for elimination of NOx . The corresponding analysis revealed that the multi-channel structure provided more surface adsorbed oxygen species and that the wall of nanotubes anchored active components efficiently, which was beneficial to improve the stability as well as dispersion of the active components. Besides, a synergistic effect between Ce and V easily occurred at the CeVTi-tube catalyst, and its reducibility was significantly improved since the electron transformation between Ce and V was dramatically enhanced. Consequently, the tailor-made multi-channel CeVTi-tube catalyst exhibited satisfied de-NOx efficiency at the temperature range of 220-460 °C. It seemed that the multi-channel TiO2 nanotubes hold great potential as an excellent carrier for SCR catalysts.
