[Pollutant Transport Analysis and Source Apportionment of the Entire Non-point Source Pollution Process in Combined...

A comprehensive and scientific understanding of non-point source pollutant transport pathways and source apportionment in combined sewer systems is essential for managing and improving the urban water environment. This study analyzed build-up and wash-off processes of pollutants on road surfaces and in sewers within a catchment of combined sewer systems in a typical old district in Zhuhai. Besides, source apportionment of the entire urban non-point source pollution was investigated by using the mass conservation method. The outcomes revealed that the build-up load of road deposited sediments in the study area was (28.81±10.69) g·m^-2. The average wash-off load of road deposited sediments during five different rainfall events was (19.27±10.90) g·m^-2 and the wash-off percentage was (52.69±13.3)%. The event mean concentrations of suspended solids (SS) in road runoff were 52-109 mg·L^-1, and the event mean concentrations of SS in sewer runoff were 68-158 mg·L^-1. Source apportionment analysis showed that road runoff, domestic wastewater, and sewer sediments contributed 39%-72%, <20%, and 13%-56% to SS, respectively. The thickness of sewer sediments increased by 1-14 cm during light and moderate rains, and the thickness decreased by 7-17 cm during heavy rains. It was found that rainfall characteristics affected the contribution percentages of pollution sources. The contribution of pollution from road runoff, domestic sewage, and sewer sediments in combined sewer systems were 2%-52%, 9%-65%, and 8%-81%, respectively. The derived outcomes should be useful for developing recommendations to control non-point source pollution in combined sewer systems and improve urban receiving water quality in China.