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Updated: Jan 1, 2026

An Analog Macroscopic Technique for Studying Molecular Hydrodynamic Processes in Dense Gases and Liquids
Published on: December 4, 2017
Daniel Jacobson1, Stephen Whitelam2
1Division of Chemistry and Chemical Engineering, California Institute of Technology, Pasadena, California 91125, USA.
This study introduces a novel importance sampling method for calculating large-deviation rate functions in continuous-time Markov chains. The technique provides tighter bounds and exact rate functions for dynamical observables without prior knowledge of rare events.
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