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Slope selection in unstable multilayer growth in 1+1 dimensions: Step flow models with downward funneling
Ian Johnson1, Christian Ratsch2, Frederic Gibou3
1Department of Mathematics, University of Maryland, College Park, Maryland 20742, USA.
This study investigates crystal growth dynamics, focusing on how step edges influence surface morphology. We found that downward funneling and step interactions lead to eventual slope selection in homoepitaxial growth.
Area of Science:
- Surface science
- Materials science
- Condensed matter physics
Background:
- Homoepitaxial crystal growth involves the deposition of material onto a crystal substrate, leading to the formation of terraces and steps.
- The dynamics of these steps are crucial for determining the final surface morphology and quality of the grown crystal.
- Understanding step dynamics is essential for controlling crystal growth and developing advanced materials.
Purpose of the Study:
- To analytically and numerically investigate the dynamics of slope selection in one-dimensional models of homoepitaxial crystal growth.
- To examine the influence of kinetic processes, including adatom diffusion, attachment/detachment kinetics, and downward funneling, on slope selection.
- To analyze the effects of boundary conditions and step-step interactions on the step flow dynamics and slope selection.
Main Methods:
- Analytical treatment using perturbation theory to characterize time-periodic solutions for slope-selected profiles.
- Numerical simulations of step flow dynamics for straight step geometries.
- Modeling of kinetic processes: adatom diffusion, Ehrlich-Schwoebel barriers, material deposition, and downward funneling (DF).
Main Results:
- Numerical simulations demonstrate that slope selection eventually occurs in the studied system.
- Perturbation theory successfully characterizes time-periodic solutions of step flow for slope-selected profiles.
- A simplified step flow theory incorporating constant probabilities for adatom motion effectively models slope selection in the presence of DF.
Conclusions:
- Slope selection is a key phenomenon in homoepitaxial crystal growth, influenced by various kinetic and interaction parameters.
- Downward funneling and repulsive step-step interactions play significant roles in achieving slope selection.
- The findings provide a framework for understanding and controlling surface morphology during crystal growth, with potential applications in materials science.
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