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Shaping electron-hole trajectories for solid-state high harmonic generation control.

Gal Orenstein, Ayelet Julie Uzan, Sagie Gadasi

    Optics Express
    |December 28, 2019
    PubMed
    Summary
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    This study introduces a monolithic scheme for solid-state high-harmonic generation (HHG) using intense infra-red (IR) laser fields. The method precisely controls the periodicity of HHG, enabling tunable extreme ultraviolet (XUV) sources.

    Area of Science:

    • Physics
    • Optics
    • Quantum Electronics

    Background:

    • Solid-state high-harmonic generation (HHG) using intense infra-red (IR) laser fields is a promising method for generating coherent attosecond light pulses in the extreme ultraviolet (XUV) spectral range.
    • Non-linear processes during IR field propagation in dense solid media significantly influence the HHG waveform.

    Purpose of the Study:

    • To introduce a monolithic scheme that leverages non-linear propagation to manipulate a two-color driving field for HHG within a single crystal.
    • To demonstrate precise control over the periodicity of the HHG process using a non-commensurate, bi-chromatic driving field.
    • To advance solid-state HHG spectroscopy and develop tunable, robust XUV sources.

    Main Methods:

    • Implementation of a monolithic scheme for simultaneous manipulation of a two-color driving field and HHG within a single crystal.

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  • Utilizing non-linear propagation effects to shape the driving laser field.
  • Employing a non-commensurate, bi-chromatic generating field to control HHG periodicity.

    • Main Results:

    • Demonstration of precise control over the periodicity of the high-harmonic generation process.
    • Ability to manipulate the spectral positions of discrete harmonic peaks.
    • Successful generation of harmonics within a single crystal using the monolithic scheme.

    Conclusions:

    • The developed monolithic scheme offers precise control over solid-state HHG by manipulating the driving field's non-linear propagation.
    • This control allows for tuning the spectral characteristics of the generated XUV light.
    • The method provides a simple and robust route towards tunable XUV sources for applications in spectroscopy and beyond.