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Active topological glass.

Jan Smrek1,2, Iurii Chubak3, Christos N Likos3

  • 1Faculty of Physics, University of Vienna, Boltzmanngasse 5, A-1090, Vienna, Austria. jan.smrek@univie.ac.at.

Nature Communications
|January 9, 2020
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Summary
This summary is machine-generated.

Researchers discovered a new glassy state in soft matter systems. This novel state arises from the interplay between active segments and circular polymer topology, impacting relaxation dynamics.

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Area of Science:

  • Soft matter physics
  • Polymer physics

Background:

  • Glass transition typically depends on packing fraction or temperature.
  • Internal particle topology's role in glassiness is conjectured but experimentally challenging.
  • Circular polymers present unique topological constraints.

Purpose of the Study:

  • To investigate the role of internal topology and activity in inducing a glassy state in soft matter.
  • To explore the relationship between polymer activity, topology, and relaxation dynamics.
  • To compare observed phenomena with biological systems like DNA in nuclei.

Main Methods:

  • Studied dense solutions of circular polymers with active segments.
  • Utilized simulations or experiments to observe the behavior of these systems.
  • Analyzed the impact of isotropic driving on polymer dynamics and relaxation.

Main Results:

  • Demonstrated that active segments in circular polymers create a novel glassy state.
  • Showed that polymer activity and topology cooperatively increase relaxation times.
  • Observed similarities between the system's dynamics and DNA fiber behavior in eukaryotic nuclei.

Conclusions:

  • Internal topology and segment activity can independently induce glassiness in soft matter.
  • The interplay between activity and topology leads to cooperative relaxation and extended timescales.
  • This model offers insights into biological phenomena like DNA organization.