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Floor- or Ceiling-Sliding for Chemically Active, Gyrotactic, Sedimenting Janus Particles.

Sayan Das1, Zohreh Jalilvand2, Mihail N Popescu1

  • 1Max-Planck-Institut für Intelligente Systeme, Heisenbergstr. 3, D-70569 Stuttgart, Germany.

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|January 29, 2020
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Summary
This summary is machine-generated.

Chemically active Janus particles exhibit sliding states near walls, influenced by gravity-driven sedimentation and self-propulsion. Their behavior, including simultaneous sliding at top and bottom surfaces, depends on sedimentation velocity and gyrotactic response.

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Area of Science:

  • Physics of active matter
  • Soft condensed matter physics
  • Colloidal science

Background:

  • Chemically active particles self-propel via surface reactions, creating chemical fields and hydrodynamic flows.
  • Interactions with confining surfaces lead to phenomena like wall-bound sliding states.
  • Janus particles, often used as model systems, are typically gyrotactic and sediment.

Purpose of the Study:

  • To theoretically investigate the occurrence of sliding states for gyrotactic, self-phoretic Janus particles near horizontal walls.
  • To quantify the influence of gravity-induced effects (sedimentation, gyrotaxis) on particle-wall interactions.
  • To construct phase diagrams mapping sliding states as a function of key physical parameters.

Main Methods:

  • Theoretical modeling of chemically active Janus particles.
  • Construction of state diagrams based on sedimentation velocity, gyrotactic response, and phoretic mobility.
  • Comparison of theoretical predictions with experimental data.

Main Results:

  • Sliding states can occur at horizontal walls (floors and ceilings).
  • Simultaneous sliding at both floor and ceiling is possible under specific conditions.
  • The parameter space reveals distinct regions for sliding at floor only, ceiling only, or no sliding states.
  • Theoretical predictions show good agreement with experimental observations.

Conclusions:

  • Gravity-induced effects significantly influence the wall-interaction behavior of active Janus particles.
  • The study provides a framework for understanding and predicting sliding states in active matter systems.
  • Experimental validation confirms the theoretical model's ability to capture complex particle dynamics near surfaces.