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Lamination of Separators to Electrodes using Electrospinning
Bernhard Christian Springer1, Martin Frankenberger1, Karl-Heinz Pettinger1
1Technology Centre for Energy, University of Applied Sciences Landshut, Ruhstorf a. d. Rott, Bavaria, Germany.
Plos One
|January 29, 2020
Summary
Electrospinning enables faster lithium-ion battery production by overcoming lamination limitations for non-thermoplastic binders. This study demonstrates successful adhesion of electrospun polymer nanofibers to battery electrodes, paving the way for advanced manufacturing.
Area of Science:
- Materials Science
- Chemical Engineering
- Electrochemistry
Background:
- Lamination is crucial for efficient lithium-ion battery (Li-ion) production, offering fast line speeds by adhering separators to electrodes.
- Current lamination technology is limited to battery components utilizing thermoplastic binders, excluding many advanced formulations.
- Overcoming binder limitations is essential for next-generation Li-ion cell manufacturing.
Purpose of the Study:
- To investigate the feasibility of Electrospinning as a viable method for advanced and rapid Li-ion cell production.
- To overcome the limitations of conventional lamination for non-thermoplastic battery materials.
- To demonstrate the successful adhesion of electrospun materials to battery electrodes.
Main Methods:
- Electrospinning of beaded polyvinylidene fluoride (PVDF) polymer nanofibers onto a fiber-reinforced, inorganic-filled separator.
- Lamination of the modified separator onto a NMC111-cathode using a specific temperature profile (110/110/120°C).
- Scanning Electron Microscopy (SEM) analysis to evaluate the adhesive behavior and successful lamination.
Main Results:
- Successful adhesion of the electrospun PVDF nanofibers to the separator was achieved.
- The modified separator demonstrated successful lamination onto the NMC111-cathode.
- SEM imaging confirmed the adhesive bonding between the polymer nanofibers and the electrode surface.
Conclusions:
- Electrospinning presents a feasible method to enhance Li-ion battery production processes.
- This technique overcomes the material constraints of traditional lamination, enabling wider applicability.
- The study confirms the potential of Electrospinning for advanced, fast-track Li-ion cell manufacturing.

