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Continuous-time quantum walk on an extended star graph: Disorder-enhanced trapping process
Saad Yalouz1, Vincent Pouthier1
1Institut UTINAM, Université de Franche-Comté, CNRS UMR 6213, 25030 Besançon Cedex, France.
Disorder in star graphs significantly enhances exciton absorption, leading to complete trapping. An optimal disorder level minimizes absorption time by restructuring exciton states, creating a superoptimized process.
Area of Science:
- Condensed matter physics
- Quantum mechanics
- Materials science
Background:
- Exciton dynamics are crucial for energy transfer in materials.
- Disorder in complex networks can significantly alter quantum phenomena.
- Star graphs provide a model for studying energy transport in branched structures.
Purpose of the Study:
- To investigate exciton dynamics on a disordered star graph with an energy-trapping central site.
- To compare the effects of disorder versus an ordered network on exciton absorption.
- To identify optimal conditions for minimizing exciton absorption time.
Main Methods:
- Utilizing a tight-binding model to simulate exciton behavior.
- Analyzing exciton dynamics on an extended star graph with a central trap.
- Comparing results from disordered and ordered network configurations.
Main Results:
- Disorder drastically improves and completes excitonic absorption compared to ordered networks.
- An optimal level of disorder is found to minimize absorption time due to exciton eigenstate restructuring.
- An optimal absorption rate further reduces trapping time, leading to a superoptimized process.
Conclusions:
- Disorder plays a critical role in enhancing and accelerating exciton trapping in star graphs.
- The interplay between disorder and superradiance transitions optimizes the energy trapping process.
- These findings have implications for designing efficient light-harvesting systems.
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