Advanced Thin Film Cathodes for Lithium Ion Batteries

Binder-free thin film cathodes have become a critical basis for advanced high-performance lithium ion batteries for lightweight device applications such as all-solid-state batteries, portable electronics, and flexible electronics. However, these thin film electrodes generally require modifications to improve the electrochemical performance. This overview summarizes the current modification approaches on thin film cathodes, where the approaches can be classified as single-phase nanostructure designs and multiphase nanocomposite designs. Recent representative advancements of different modification approaches are also highlighted. Besides, this review discusses the existing challenges regarding the thin film cathodes. The review also discusses the future research directions and needs towards future advancement in thin film cathode designs for energy storage needs in advanced portable and personal electronics.