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Updated: Dec 26, 2025

Methods of Ex Situ and In Situ Investigations of Structural Transformations: The Case of Crystallization of Metallic Glasses
Published on: June 7, 2018
Spin-Orbital Glass Transition in a Model of a Frustrated Pyrochlore Magnet without Quenched Disorder
Kota Mitsumoto1, Chisa Hotta2, Hajime Yoshino1,3
1Graduate School of Science, Osaka University, Toyonaka, Osaka 560-0043, Japan.
Abstract:
We show theoretically that spin and orbital degrees of freedom in the pyrochlore oxide Y_{2}Mo_{2}O_{7}, which is free of quenched disorder, can exhibit a simultaneous glass transition, working as dynamical disorder for each other. The interplay of spins and orbitals is mediated by the Jahn-Teller lattice distortion that selects the choice of orbitals, which then generates variant spin exchange interactions ranging from ferromagnetic to antiferromagnetic ones. Our Monte Carlo simulations detect the power-law divergence of the relaxation times and the negative divergence of both the magnetic and dielectric nonlinear susceptibilities, resolving the long-standing puzzle on the origin of the disorder-free spin glass.
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