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Updated: Dec 25, 2025

Direct Imaging of Laser-driven Ultrafast Molecular Rotation
Published on: February 4, 2017
Rotation-sensitive and direction-resolved homodyne laser-Doppler vibrometry method for simultaneous measurement of
Abstract:
In this paper, we introduce a new rotation-sensitive and direction-resolved homodyne laser-Doppler vibrometry method for rigid body vibration study that is based on the discrete Fourier-transform of successive 1D profiles of the moving interference fringes recorded with a 1D array detector. By investigating the temporal evolution of the spatial phase distribution of the 1D profiles of the interference fringes, the out-of-plane translational and rotational vibrations of the vibrating object are simultaneously determined. We use a direction-cosine-based approach to establish the theory of the measurements. The merits and limitations of the proposed method is described. We show that the proposed method can be used for detection of both tip and tilt changes and out-of-plane displacement measurements of a rigid body using a couple of parallel 1D array detectors. In addition, we show that the presented method can be also used on optical diffused surfaces by adding three lenses in a corner-like arrangement to the detecting system.
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