Dynamic photonic crystal in a colloidal quantum-dot solution: formation, structure analysis, and dimensionality...

We demonstrated, for the first time, to the best of our knowledge, a simple method to create three-dimensional (3D) dynamic photonic crystal (PhC) with controllable lattice symmetry through the interference of four non-coplanar laser beams in a non-linear optical medium [colloidal solution of CdSe/ZnS quantum dots (QDs)]. 3D dynamic PhC was formed due to the periodically changing refraction and absorption of resonantly excited excitons in the colloidal solution of QDs. The formation of dynamic PhC was confirmed by the observed self-diffraction of the laser beams on the dynamic structure which they have created. Tuning of the PhC dimensionality to the two-dimensional (2D) and one-dimensional (1D) was done through the reduction of the number of interfering beams to three and two, respectively, and by controlling the polarization of interacting beams. Physical processes responsible for the observed self-action effects that arise in CdSe/ZnS QDs are discussed in detail.