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Synthesis of Non-uniformly Pr-doped SrTiO3 Ceramics and Their Thermoelectric Properties

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Published on: August 15, 2015

Specific heat of single-crystal PrMnO₃.

J G Cheng¹, Y Sui, X J Wang

¹Center for Condensed Matter Science and Technology (CCMST), Department of Applied Physics, Harbin Institute of Technology, Harbin 150001, People's Republic of China.

Journal of Physics. Condensed Matter : an Institute of Physics Journal

|May 14, 2020

Summary

This study measured the specific heat of PrMnO3 under magnetic fields, revealing details about magnetic ordering and energy levels. Magnetic fields influence spin fluctuations and the antiferromagnetic transition temperature.

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Area of Science:

Condensed Matter Physics
Magnetism
Thermodynamics

Background:

Praseodymium manganite (PrMnO3) is a material exhibiting complex magnetic properties.
Understanding the interplay between crystal structure, magnetic ordering, and external fields is crucial for materials science.

Purpose of the Study:

To investigate the specific heat of single-crystal PrMnO3 across a range of temperatures (2-200 K) and magnetic fields (up to 8 T).
To determine the energy levels of Pr3+ ions and analyze the magnetic ordering of Mn3+ spins under varying magnetic conditions.

Main Methods:

Specific heat measurements were performed on single-crystal PrMnO3 from 2 to 200 K.
Analysis involved fitting the specific heat data to determine Pr3+ energy levels and magnetic contributions.
Magnetic entropy was calculated by subtracting lattice and Pr3+ contributions.

Main Results:

A Schottky-like anomaly, attributed to Pr3+ ions, shifted to higher temperatures with increasing magnetic fields.
The first four energy singlets of the Pr3+ 3H4 ground multiplet were determined.
The Pr-Mn exchange field was found to be negligible.
The antiferromagnetic ordering of Mn3+ spins (at TN) showed a lambda-shaped anomaly, which was suppressed and broadened by magnetic fields.
Magnetic entropy above TN increased with field strength due to enhanced spin fluctuations.

Conclusions:

The study provides a detailed characterization of the magnetic phase transitions and energy level structure in PrMnO3.
Magnetic fields significantly influence spin dynamics and the cooperative antiferromagnetic ordering of Mn3+ spins.
The negligible Pr-Mn exchange field is consistent with the observed magnetic anisotropy of Pr3+ ions.