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Related Experiment Video

Updated: Dec 21, 2025

Scalable Syntheses of Graphene Oxide and Reduced Graphene Oxide using Cascade Design Oxidation and Highly Basic Reduction Reactions
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Scalable Syntheses of Graphene Oxide and Reduced Graphene Oxide using Cascade Design Oxidation and Highly Basic Reduction Reactions

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Doping effect in graphene-graphene oxide interlayer.

Mohd Musaib Haidari1, Hakseong Kim2, Jin Hong Kim1

  • 1Department of Physics, Konkuk University, Seoul, 05029, Korea.

Scientific Reports
|May 20, 2020
PubMed
Summary

Graphene oxide effectively p-dopes graphene in van der Waals heterostructures, enhancing optical and electrical properties for advanced electronic devices.

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Area of Science:

  • Materials Science
  • Condensed Matter Physics
  • Nanotechnology

Background:

  • Interlayer coupling in van der Waals (vdW) heterostructures significantly influences physical properties.
  • Understanding these interactions is crucial for developing next-generation electronic and opto-electronic devices.

Purpose of the Study:

  • To investigate the optical and electrical properties of a graphene/graphene oxide heterostructure.
  • To determine the doping effects and interlayer interactions within this vdW heterostructure.

Main Methods:

  • Fabrication of a vertically stacked large-area heterostructure: monolayer graphene on monolayer graphene oxide.
  • Characterization using Raman spectroscopy.
  • Density functional theory (DFT) calculations for charge transport analysis.

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Last Updated: Dec 21, 2025

Scalable Syntheses of Graphene Oxide and Reduced Graphene Oxide using Cascade Design Oxidation and Highly Basic Reduction Reactions
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Main Results:

  • The graphene/graphene oxide heterostructure exhibits effective and stable p-doping.
  • Sustainable p-doping effects are observed in graphene due to the underlying graphene oxide, despite weak interlayer interactions.
  • The p-doping is more pronounced compared to graphene on a silicon oxide substrate.

Conclusions:

  • The study demonstrates controllable p-doping in graphene via graphene oxide in vdW heterostructures.
  • This finding supports the development of novel graphene-based heterostructures for advanced functionalities.
  • Potential for enhanced applications in integrated electronic and opto-electronic devices.