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Beyond Frameworks: Structuring Reticular Materials across Nano-, Meso-, and Bulk Regimes.

Frederik Haase1, Patrick Hirschle2, Ralph Freund2

  • 1Institute for Integrated Cell-Material Sciences (WPI-iCeMS), Kyoto University, Yoshida, Sakyo-ku, Kyoto, 606-8501, Japan.

Angewandte Chemie (International Ed. in English)
|May 26, 2020
PubMed
Summary

Reticular materials offer diverse applications but require advanced structuring. This review explores self-assembly and external tools for manufacturing these materials across all scales, enabling societal impact.

Keywords:
covalent organic frameworksexternal controlmetal-organic frameworksnanoparticlesself-assembly

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Area of Science:

  • Materials Science
  • Nanotechnology
  • Chemical Engineering

Background:

  • Reticular materials, with their open, extended frameworks, are crucial for catalysis, separation, gas storage, and drug delivery.
  • Tailoring crystal structures enables specific applications, but interfacing molecular-level functionality with the macroscopic world remains a challenge.

Purpose of the Study:

  • To review recent advances in manufacturing reticular materials across multiple length scales.
  • To highlight the importance of structural control from molecular to bulk regimes.
  • To explore the use of self-assembly and externally controlled tools for material fabrication.

Main Methods:

  • Overview of self-assembly techniques for reticular material synthesis.
  • Discussion of externally controlled manufacturing tools for structured materials.
  • Analysis of methods for achieving structural control across molecular, nano-, meso-, and bulk scales.

Main Results:

  • Self-assembly and external tools are effective for manufacturing reticular materials at various scales.
  • Progress has been made in bridging the gap between molecular design and macroscopic implementation.
  • Successful structuring across length scales is key to unlocking material potential.

Conclusions:

  • Advancements in self-assembly and external manufacturing tools are critical for reticular materials.
  • Overcoming structuring barriers will enable wider application of these materials.
  • Future research in these areas will facilitate societal problem-solving.