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Screening of Coatings for an All-Solid-State Battery Using In Situ Transmission Electron Microscopy
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Passivation of the Cathode-Electrolyte Interface for 5 V-Class All-Solid-State Batteries.

Gaozhan Liu1,2, Yong Lu3, Hongli Wan1,2

  • 1Ningbo Institute of Materials Technology and Engineering, Chinese Academy of Sciences, Ningbo 315201, P. R. China.

ACS Applied Materials & Interfaces
|May 28, 2020
PubMed
Summary

Researchers developed a new all-solid-state battery using a coated cathode material. This strategy stabilizes interfaces and improves performance for advanced energy storage applications.

Keywords:
5 V-class all-solid-state batteriesInterfacial passivationLi6PS5ClLiNbO3-coatingLiNi0.5Mn1.5O4 cathode

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Area of Science:

  • Materials Science
  • Electrochemistry
  • Energy Storage

Background:

  • All-solid-state batteries offer advantages over lithium-ion batteries in safety, energy density, and operating conditions.
  • Developing stable interfaces between cathode and solid electrolyte materials is crucial for high-performance solid-state batteries.

Purpose of the Study:

  • To enhance the stability of the interface between a 5 V-class spinel LiNi0.5Mn1.5O4 (LNMO) cathode and a Li6PS5Cl (LPSCl) solid electrolyte.
  • To suppress detrimental side reactions and improve the electrochemical performance of all-solid-state batteries.

Main Methods:

  • A wet-chemistry approach was used to decorate LNMO particles with oxide materials (LiNbO3, Li3PO4, Li4Ti5O12).
  • Electrochemical characterization was performed to evaluate the performance of the modified LNMO-LPSCl composite cathodes.

Main Results:

  • The composite cathode with 8 wt% LiNbO3-coated LNMO and LPSCl (70:30 ratio) showed the best performance.
  • An initial discharge capacity of 115 mA h g-1 and a reversible capacity of 80 mA h g-1 at the 20th cycle were achieved.

Conclusions:

  • Interfacial passivation using oxide coatings is an effective strategy for stabilizing 5 V-class all-solid-state batteries.
  • The developed LNMO-based composite cathode demonstrates potential for high-performance energy storage.