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Pressure-Dependent Intermediate Magnetic Phase in Thin Fe3GeTe2 Flakes.
Heshen Wang1,2, Runzhang Xu3, Cai Liu2
1School of Electronics and Information Technology, Sun Yat-Sen University, Guangzhou 510275, P. R. China.
Ferromagnetism in Fe3GeTe2 flakes evolves under pressure, showing a new intermediate state above 7 GPa. This transition impacts magnetic properties and domain structure, offering insights into layered magnetic materials.
Area of Science:
- Condensed Matter Physics
- Materials Science
- Magnetism
Background:
- Layered magnetic materials like Fe3GeTe2 are promising for spintronic applications.
- Understanding their magnetic properties under external stimuli is crucial for device development.
Purpose of the Study:
- To investigate the pressure- and temperature-dependent evolution of ferromagnetism in Fe3GeTe2.
- To elucidate the nature of magnetic phase transitions and their underlying mechanisms.
Main Methods:
- In situ magnetic circular dichroism (MCD) spectroscopy was employed to probe magnetic behavior.
- High-pressure experiments were conducted using specialized equipment.
- First-principles calculations were performed to complement experimental findings.
Main Results:
- A rectangular hysteresis loop was observed below 7 GPa, transitioning to an intermediate, skewed loop above this pressure.
- Coercive field and Curie temperature decreased with increasing pressure, indicating reduced exchange interaction and anisotropy.
- A labyrinthine domain structure was identified in the intermediate phase, explained by Jagla's theory.
- A weak structural transition around 6 GPa correlated with changes in Fe-Fe bond length and magnetic interactions.
Conclusions:
- Pressure significantly alters the magnetic properties and phase behavior of Fe3GeTe2.
- The observed intermediate magnetic state is linked to a delicate balance between exchange interaction and magneto-crystalline anisotropy.
- Structural changes play a critical role in modulating magnetic interactions in this layered material.
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