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Highly energy-tunable quantum light from moiré-trapped excitons.

H Baek1, M Brotons-Gisbert2, Z X Koong2

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We demonstrate quantum light emission from single moiré-trapped excitons in 2D semiconductors. This confirms their quantum nature and enables tuning for quantum technologies.

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Area of Science:

  • Quantum optics
  • Condensed matter physics
  • Materials science

Background:

  • Photon antibunching signifies quantum light emission from single emitters.
  • Two-dimensional (2D) semiconductor heterostructures offer potential for novel quantum light sources.
  • Moiré potentials in 2D materials are predicted to host arrays of quantum emitters, but their quantum nature requires confirmation.

Purpose of the Study:

  • To confirm the quantum nature of moiré-trapped excitons in 2D semiconductor heterostructures.
  • To investigate the optical properties and tunability of these moiré-confined excitons.

Main Methods:

  • Photon correlation measurements to observe photon antibunching.
  • Magneto-optical spectroscopy to analyze exciton spectra.
  • Direct current (DC) Stark tuning to assess exciton energy manipulation.

Main Results:

  • Observed photon antibunching from single moiré-trapped interlayer excitons, confirming quantum emission.
  • Demonstrated discrete anharmonic spectra attributed to excitons confined in moiré potentials.
  • Achieved significant DC Stark tuning (up to 40 meV) due to the large exciton dipole moment.

Conclusions:

  • Moiré-confined excitons in 2D heterostructures exhibit quantum light emission.
  • These quantum emitters can be tuned using electric fields, opening avenues for quantum applications.
  • Further research can explore emitter inhomogeneity and interactions for advanced quantum devices.