Spin dynamics at interfaces on femtosecond timescales

The excitation of magnetically ordered materials with ultrashort laser pulses results in magnetization dynamics on femto- to picosecond timescales. These non-equilibrium spin dynamics have emerged as a rapidly developing research field in recent years. Unraveling the fundamental microscopic processes in the interaction of ultrashort optical pulses with the charge, spin, orbital, and lattice degrees of freedom in magnetic materials shows the potential for controlling spin dynamics on their intrinsic timescales and thereby bring spintronics applications into the femtosecond range. In particular, femtosecond spin currents offer fascinating new possibilities to manipulate magnetization in an ultrafast and non-local manner, via spin injection and spin transfer torque at the interfaces of ferromagnetic layered structures. This topical review covers recent progress on spin dynamics at interfaces on femtosecond time scales. The development of the field of ultrafast spin dynamics in ferromagnetic heterostructures will be reviewed, starting from spin currents propagating on nanometer length scales through layered structures before focusing on femtosecond spin transfer at interfaces. The properties of these ultrafast spin-dependent charge currents will be discussed, as well as the materials dependence of femtosecond spin injection, the role of the interface properties, and competing microscopic processes leading to a loss of spin polarization on sub-picosecond timescales.