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Updated: Dec 6, 2025

Designed for Molecular Recycling: A Lignin-Derived Semi-aromatic Biobased Polymer
Published on: November 30, 2020
Recycling of a Biodegradable Polymer Blend
Francesco Paolo La Mantia1,2, Luigi Botta1,2, Maria Chiara Mistretta1
1Department of Engineering, University of Palermo, Viale delle Scienze, 90128 Palermo, Italy.
Mechanical recycling of poly(butylene adipate-co-terephthalate) (PBAT) blends shows less property degradation when processed dry versus wet. Despite some property loss, PBAT blends can be reused after multiple extrusion cycles.
Area of Science:
- Materials Science
- Polymer Science
- Sustainable Materials
Background:
- Mechanical recycling is crucial for enhancing the value of postconsumer plastics.
- Recycled plastic performance depends on material selection and property degradation during reprocessing.
Purpose of the Study:
- To investigate the impact of five successive extrusion cycles on PBAT blend properties.
- To compare the effects of dry versus wet reprocessing conditions on material performance.
Main Methods:
- Reprocessing of a poly(butylene adipate-co-terephthalate) (PBAT)-based blend through five extrusion cycles.
- Evaluation of rheological, mechanical, and thermal properties.
- Comparison of samples processed under dry and wet conditions.
Main Results:
- Dry reprocessing resulted in less material degradation compared to wet reprocessing.
- Significant decreases in rheological and mechanical properties were observed in both conditions.
- The PBAT blend retained usable properties even after multiple reprocessing cycles.
Conclusions:
- PBAT-based blends exhibit resilience to mechanical recycling, with dry processing being preferable.
- The material's properties, while reduced, remain viable for reuse, supporting circular economy principles.
- Further research can optimize recycling processes to minimize property loss in PBAT blends.
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