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Direct electron-beam patterning of monolayer MoS2 with ice
Guangnan Yao1, Ding Zhao, Yu Hong
1College of Optical Science and Engineering, Zhejiang University, Hangzhou 310027, China.
Nanoscale
|November 9, 2020
Summary
We developed a novel ice-assisted electron-beam patterning technique for monolayer molybdenum disulfide (MoS2), achieving sub-30 nm nanoribbons without resist contamination. This contamination-free method offers a promising route for fabricating advanced two-dimensional (2D) material devices.
Area of Science:
- Materials Science
- Nanotechnology
- Condensed Matter Physics
Background:
- Two-dimensional transition metal dichalcogenides (TMDCs) are promising next-generation semiconductor materials.
- Conventional nanofabrication methods often involve resist contamination, limiting device performance.
- Developing clean and precise patterning techniques for 2D materials is crucial.
Purpose of the Study:
- To introduce a novel, contamination-free electron-beam patterning method for monolayer MoS2.
- To investigate the influence of electron beam parameters on patterning resolution.
- To demonstrate the potential for fabricating nanoscale devices using this technique.
Main Methods:
- Direct electron-beam patterning of monolayer MoS2.
- Utilizing an ice lithography-inspired approach for in situ processing.
- Systematic variation of electron beam dose and energy.
Main Results:
- Achieved direct patterning of monolayer MoS2 without polymer resist contamination.
- Fabricated nanoribbons with widths below 30 nm.
- Demonstrated the tunability of patterning resolution via electron beam parameters.
Conclusions:
- Ice-assisted electron-beam patterning is a viable, contamination-free technique for MoS2 nanofabrication.
- This method is adaptable for other TMDCs, enabling versatile 2D material device fabrication.
- Offers a promising alternative for high-performance nanoscale electronic devices.

