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Updated: Nov 29, 2025

Photoelectron Imaging of Anions Illustrated by 310 Nm Detachment of F−
Published on: July 27, 2018
Time-resolved dissociative ionization and double photoionization of CO2
Dror M Bittner1, Krishnendu Gope1, Daniel Strasser1
1Institute of Chemistry, The Hebrew University of Jerusalem, Jerusalem 9190401, Israel.
Abstract:
CO2 single-photon double photoionization, Coulomb explosion, and dissociative ionization are studied with ultrafast extreme-ultraviolet pump and time-delayed near-infrared probe pulses. Kinetic energy release and momentum correlations for the two-body CO+ + O+ and three-body O+ + C+ + O fragmentation products are determined by 3D coincidence fragment imaging. The transient enhancement of the ratio of two-body vs three-body Coulomb explosion events and the time dependence of low and high kinetic energy release dissociation events are discussed in terms of dissociative ionization and Coulomb explosion dynamics.
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