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Phase Inversion-Based Technique for Fabricating Bijels and Bijels-Derived Structures with Tunable Microstructures.

Junzhi Li1, Haoran Sun1, Min Wang1

  • 1Department of Mechanical Engineering, The University of Hong Kong, Pokfulam Road, Hong Kong, China.

Langmuir : the ACS Journal of Surfaces and Colloids
|November 25, 2020
PubMed
Summary
This summary is machine-generated.

A new phase inversion technique enables the fabrication of bicontinuous interfacially jammed emulsion gels (bijels) and their derived structures. This method allows control over bijel properties and drug release from hybrid hydrogels for biomedical applications.

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Area of Science:

  • Soft matter physics
  • Materials science
  • Biomedical engineering

Background:

  • Bicontinuous interfacially jammed emulsion gels (bijels) are advanced soft materials with two continuous phases.
  • Fabrication challenges and structural control limit bijel applications.
  • Bijels offer potential in diverse fields, including biomedicine.

Purpose of the Study:

  • Develop a facile and reproducible method for fabricating bijels and bijel-derived structures.
  • Investigate the influence of casting solution composition on bijel properties.
  • Explore the controlled release of drugs from bijel-derived hybrid hydrogels.

Main Methods:

  • Phase inversion technique for bijel fabrication.
  • Compositional variation of casting solutions.
  • Fabrication of composite bijels using two organic monomers.
  • Loading and in vitro release studies of doxorubicin hydrochloride (DOX).
  • In vitro degradation studies of alginate-based hybrid hydrogels.

Main Results:

  • The phase inversion method successfully produced bijels with tunable porosity, oil-to-water ratio, and domain size.
  • Incorporating a second monomer offered further control over bijel structure.
  • Bijel-derived hybrid hydrogels successfully encapsulated and controlled the release of DOX.
  • Alginate cross-linking regulated hydrogel degradation and drug release kinetics.

Conclusions:

  • A robust protocol for controlled bijel fabrication was established.
  • The technique facilitates the creation of bijel-derived structures for biomedical applications.
  • This work paves the way for advanced drug delivery systems using bijel technology.