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Self-Assembled Periodic Nanostructures Using Martensitic Phase Transformations.

Abhinav Prakash1, Tianqi Wang1, Ashley Bucsek2,3

  • 1Department of Chemical Engineering and Materials Science, University of Minnesota, Twin Cities, Minneapolis, Minnesota 55455, United States.

Nano Letters
|December 2, 2020
PubMed
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Researchers developed a new method for creating self-assembled nanostructures using martensitic phase transformations. This technique allows for tunable, reconfigurable periodic nanostructures in strontium tin oxide (SrSnO3) thin films for optoelectronic applications.

Area of Science:

  • Materials Science
  • Nanotechnology
  • Condensed Matter Physics

Background:

  • Periodic nanostructures are crucial for advanced optoelectronic devices.
  • Existing fabrication methods often lack scalability and tunability.

Purpose of the Study:

  • To present a novel approach for designing and synthesizing self-assembled periodic nanostructures.
  • To demonstrate the use of martensitic phase transformations for creating reconfigurable nanostructures.

Main Methods:

  • Utilized martensitic phase transformations in perovskite SrSnO3 thin films.
  • Employed chemical doping and strain engineering to control periodicity and phase fractions.
  • Tuned dielectric contrast using temperature and laser wavelength.
Keywords:
Phase transformationmetamaterialsmolecular beam epitaxynanostructureself-assemblysemiconductor

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Main Results:

  • Successfully created reconfigurable periodic nanostructures with sharply contrasted dielectric properties.
  • Achieved tunable periodicity and relative phase fractions.
  • Demonstrated the potential for creating variable photonic crystals.

Conclusions:

  • Martensitic phase transformations offer a viable route for large-area, self-assembled periodic nanostructures.
  • This approach enables the design of "built-to-order" nanostructures for tailored optoelectronic functionalities.