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Updated: Nov 23, 2025

Direct Imaging of Laser-driven Ultrafast Molecular Rotation
Published on: February 4, 2017
Ultraviolet intracavity frequency-doubled Pr3+:LiYF4 orbital Poincaré laser
Abstract:
Here we demonstrate intracavity frequency-doubling of an ultra-compact (cavity length < 20 mm) Pr3+:LiYF4 (YLF) orbital Poincaré laser, in which the fundamental modes are represented on an equivalent orbital Poincaré sphere (eOPS) and a singularities hybrid evolution nature sphere (SHENS). The generated ultraviolet (UV, 320 nm) output carries orbital angular momentum (OAM), and it typically exhibits an optical bottle beam with a 3-dimensional dark core, formed of a coherent superposition of eigen Laguerre-Gaussian (LG) modes. Such ultraviolet structured light beams with OAM offer many advanced applications from microscopy to materials processing.

