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We present a theory for optical and transport properties of molecular junctions using Floquet theory and nonequilibrium Green's functions. This work advances understanding of periodically driven quantum systems for quantum technologies.

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Area of Science:

  • Quantum physics
  • Materials science
  • Nanotechnology

Background:

  • Optical control of matter is crucial for fundamental insights and technological applications.
  • Theoretical modeling of periodically driven systems is essential for developing nanoscale quantum devices.
  • Understanding open quantum systems under external driving is key to advancing quantum technologies.

Purpose of the Study:

  • To develop a theoretical framework for analyzing the transport and optical response of molecular junctions under periodic driving.
  • To investigate the influence of external periodic driving on the behavior of open nonequilibrium quantum systems.
  • To provide a foundation for engineering quantum devices utilizing light-matter interactions.

Main Methods:

  • Utilizing Floquet theory to describe periodic driving.
  • Employing nonequilibrium Green's function formalism for open quantum systems.
  • Applying the self-consistent Born approximation to model light-matter interactions.
  • Using a generic three-level model for illustration.

Main Results:

  • A theoretical model for transport and optical response in periodically driven molecular junctions has been developed.
  • The study illustrates how periodic driving affects the optical and transport properties of these systems.
  • The findings provide insights into controlling quantum phenomena in nanoscale devices.

Conclusions:

  • The developed theory offers a pathway to characterize and control matter using optical means in molecular junctions.
  • This research contributes to the fundamental understanding of periodically driven quantum systems.
  • The work has implications for the design and development of future quantum technologies.