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Updated: Nov 18, 2025

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Published on: March 30, 2017
Ultrafast control of magnetic interactions via light-driven phonons
D Afanasiev1, J R Hortensius2, B A Ivanov3,4
1Kavli Institute of Nanoscience, Delft University of Technology, Delft, the Netherlands. dmytro.afanasiev@physik.uni-regensburg.de.
Researchers used light-driven phonons to control magnetic states in antiferromagnets. This technique allows for ultrafast switching between different magnetic orders, opening new avenues for materials science.
Area of Science:
- Condensed Matter Physics
- Materials Science
- Ultrafast Spectroscopy
Background:
- Resonant excitation of infrared-active phonons is a key method for controlling material electronic properties.
- Previous studies demonstrated light-induced superconductivity, ferroelectric polarization switching, and insulator-to-metal transitions.
- Macroscopic magnetic states are typically controlled by external magnetic fields or temperature.
Purpose of the Study:
- To investigate the potential of light-driven phonons for coherent manipulation of macroscopic magnetic states.
- To explore non-thermal lattice control of magnetic exchange interactions.
- To achieve ultrafast switching between competing magnetic orders.
Main Methods:
- Intense mid-infrared electric field pulses were used for resonant excitation of phonon modes.
- The archetypal antiferromagnet DyFeO3 was used as the model material.
- Time-resolved measurements were employed to observe changes in magnetic exchange interactions and spin orders.
Main Results:
- Ultrafast and long-living changes in the exchange interaction between rare-earth orbitals and transition metal spins were induced.
- Coherent switching between antiferromagnetic and weakly ferromagnetic spin orders was achieved on picosecond timescales.
- Non-thermal lattice control of magnetic exchange was demonstrated.
Conclusions:
- Light-driven phonons can be utilized to coherently manipulate macroscopic magnetic states.
- Resonant phonon excitation offers a powerful tool for ultrafast control of ferroic order.
- This discovery opens new possibilities for designing and controlling magnetic materials.
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