Low-energy magnons in the chiral ferrimagnet Cu₂OSeO₃: A coarse-grained approach

We report a comprehensive neutron scattering study of low energy magnetic excitations in the breathing pyrochlore helimagnetic Cu₂OSeO₃. Fully documenting the four lowest energy magnetic modes that leave the ferrimagnetic configuration of the "strong tetrahedra" intact ( $\left|\hslash \omega \right|<13$ meV), we find gapless quadratic dispersion at the point for energies above 0.2 meV, two doublets separated by 1.6(2) meV at the R point, and a bounded continuum at the X point. Our constrained rigid spin cluster model relates these features to Dzyaloshinskii-Moriya (DM) interactions and the incommensurate helical ground state. Combining conventional spin wave theory with a spin cluster form factor accurately reproduces the measured equal time structure factor through multiple Brillouin zones. An effective spin Hamiltonian describing complex anisotropic intercluster interactions is obtained.