Approaching Single-Photon Pulses

Single-photon pulses cannot be generated on demand, due to incompatible requirements of positive frequencies and positive times. Resulting states therefore contain small probabilities for multiphotons. We derive upper and lower bounds for the maximum fidelity of realizable states that approximate single-photon pulses. The bounds have implications for ultrafast optics; the maximum fidelity is low for pulses with few cycles or close to the onset, but increases rapidly as the pulse envelope varies more slowly. We also demonstrate strictly localized states that are close to single photons.