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Updated: Nov 12, 2025

Ultrafast Time-resolved Near-IR Stimulated Raman Measurements of Functional π-conjugate Systems
Published on: February 10, 2020
Detection of photon statistics and multimode field correlations by Raman processes
Frank Schlawin1, Konstantin E Dorfman2, Shaul Mukamel3
1The Hamburg Centre for Ultrafast Imaging, Luruper Chaussee 149, 22761 Hamburg, Germany.
Abstract:
Glauber's g(2)-function provides a common measure of quantum field statistics through two-photon coincidence counting in Hanbury Brown-Twiss measurements. Here, we propose to use nonlinear optical signals as a tool for the characterization of quantum light. In particular, we show that Raman measurements provide an alternative direct probe for a different component of the four-point correlation function underlying the g(2)-function. We illustrate this capacity for a specific quantum state obtained from a frequency conversion process. Our work points out how the analysis of controlled optical nonlinear processes can provide an alternative window toward the analysis of quantum light sources.
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