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Crystalline Porous Materials for Nonlinear Optics.

Rongchao Shi1, Xiao Han1, Jialiang Xu1

  • 1School of Materials Science and Engineering, National Institute for Advanced Materials, Nankai University, Tongyan Road 38, Tianjin, 300350, P. R. China.

Small (Weinheim an Der Bergstrasse, Germany)
|March 18, 2021
PubMed
Summary

Crystalline porous materials offer tunable structures for advanced nonlinear optics (NLO) applications. This review highlights recent progress in NLO materials, focusing on second- and third-order effects for diverse applications.

Keywords:
covalent organic frameworkscrystalline porous materialsmetal-organic frameworksnonlinear opticspolyoxometalates

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Area of Science:

  • Materials Science
  • Optics
  • Chemistry

Background:

  • Crystalline porous materials, including metal-organic frameworks (MOFs), covalent organic frameworks (COFs), and polyoxometalates, are versatile platforms.
  • Their unique structures allow for precise organization and modification of chromophores, crucial for nonlinear optical (NLO) properties.
  • These materials have broad applications in frequency doubling, two-photon absorption/emission, optical limiting, photoelectric conversion, and bioimaging.

Purpose of the Study:

  • To review recent advancements in crystalline porous materials designed for nonlinear optical (NLO) applications.
  • To discuss the classification and characteristics of second- and third-order NLO crystalline porous materials.
  • To highlight key properties, applications, and future research directions in this field.

Main Methods:

  • Literature review of recent research on crystalline porous nonlinear optical materials.
  • Categorization of second-order NLO materials based on chiral and achiral structures.
  • Classification of third-order NLO materials into pure organic and hybrid organic/inorganic types.

Main Results:

  • Recent progress in crystalline porous materials for NLO applications has been discussed.
  • Second-order NLO materials primarily focus on chiral and achiral structures.
  • Third-order NLO materials are categorized into pure organic and hybrid organic/inorganic systems, with representative properties and applications highlighted.

Conclusions:

  • Crystalline porous materials provide excellent platforms for developing advanced NLO materials due to their structural tunability.
  • Significant progress has been made in both second- and third-order NLO applications.
  • Future research should address challenges and explore new directions for enhanced NLO performance and broader applications.