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Highly Efficient Thermal Energy Storage Using a Hybrid Hypercrosslinked Polymer*.

Changhui Liu1, Jiahao Zhang1, Jian Liu1

  • 1School of Electrical and Power Engineering, China University of Mining and Technology, Xuzhou, Jiangsu, 221116, China.

Angewandte Chemie (International Ed. in English)
|April 2, 2021
PubMed
Summary
This summary is machine-generated.

A novel hybrid polymer effectively encapsulates phase change materials (PCMs), enhancing thermal conductivity by 600% and achieving high light-to-thermal conversion. This method also imparts self-cleaning properties to the PCMs.

Keywords:
energy storagehybrid materialsphase change materialsphase transitionsself-cleaning

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Area of Science:

  • Materials Science
  • Polymer Chemistry

Background:

  • Phase change materials (PCMs) are crucial for thermal energy storage but often suffer from leakage and poor thermal conductivity.
  • Developing effective encapsulation methods is essential to overcome these limitations and enhance PCM performance.

Purpose of the Study:

  • To synthesize an organic/inorganic hybrid polymer for encapsulating phase change materials (PCMs).
  • To improve the thermal conductivity and light-to-thermal conversion efficiency of PCMs.
  • To investigate the self-cleaning properties imparted by the hybrid polymer encapsulation.

Main Methods:

  • Synthesis of a siloxyl-functionalized organic/inorganic hybrid polymer via a mild hypercrosslinking reaction.
  • Encapsulation of both organic and inorganic PCMs within the hybrid polymer matrix.
  • Incorporation of nano-additives for thermal conductivity enhancement.

Main Results:

  • Achieved a 600% enhancement in thermal conductivity.
  • Reached 93.7% light-to-thermal conversion efficiency.
  • Demonstrated a latent heat of 180 J/g with no leakage and notable self-cleaning properties.
  • Successfully encapsulated various nanoparticles, including carbon-based and metal oxide nanomaterials.

Conclusions:

  • The developed hybrid polymer provides an effective and versatile method for PCM encapsulation.
  • The encapsulation enhances thermal properties and introduces self-cleaning capabilities.
  • This approach is suitable for advanced thermal energy storage applications.