The level, distribution and source of artificial radionuclides in surface soil from Inner Mongolia, China

Mid- and long-half-life artificial radioisotopes in the earth's surface environment are of great concern to the environmental radiation risk assessment. As nuclear fuel and fission products, ²³⁹Pu, ²⁴⁰Pu, ²⁴¹Am, ⁹⁰Sr and ¹³⁷Cs in soils from Inner Mongolia of China were analyzed with a modified systematic separation procedure combined with ICP-MS and LSC measurements, to study the level, distribution and source of artificial radionuclides in the region. The radioactivity and inventory of ¹³⁷Cs (0.26-28.3 Bq/kg, 0.5-5.4 kBq/m²), ^239+240Pu (0.05-1.26 Bq/kg, 20-229 Bq/m²), ²⁴¹Am (0.036-0.35 Bq/kg, 11-81 Bq/m²) and ⁹⁰Sr (1.2-7.6 Bq/kg, 0.39-1.7 kBq/m²) all lie in the range of the global fallout. Vertical distributions of these radionuclides were examined for two soil core samples SC14025 and SC14038, and great differences were observed between these two sample locations. For SC14025 where little human disturbance to soil occurred, both ¹³⁷Cs and ^239+240Pu have a subsurface activity maximum followed by an exponential decay. Fittings base on CDE model gives a small downward migration velocity of about 0.097 cm/y for both Pu and ¹³⁷Cs. Source identification for SC14025 and SC14038 soil cores with ²⁴⁰Pu/²³⁹Pu (average of 0.180 ± 0.017 and 0.164 ± 0.035, respectively), ¹³⁷Cs/^239+240Pu (average of 25.3 ± 0.6 and 25.6 ± 3.0, respectively) and ²⁴¹Am/^239+240Pu (average of 0.56 ± 0.08 and 0.60 ± 0.09, respectively) ratios consistently indicated that anthropogenic radionuclides in Xilingol region are mostly from the global fallout of atmospheric nuclear weapons tests in the last century. According to the geographical distribution of the radioactivity level, the high radioactivity level in the east of Inner Mongolia probably results from enhanced deposition by the blocking of the Great Khingan Range.