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Materials Design and Optimization for Next-Generation Solar Cell and Light-Emitting Technologies.

Sergei Manzhos¹, Chu-Chen Chueh^2,3, Giacomo Giorgi^4,5

¹School of Materials and Chemical Technology, Tokyo Institute of Technology, Ookayama 2-12-1, Meguro-ku, Tokyo 152-8552, Japan.

The Journal of Physical Chemistry Letters

|May 11, 2021

Summary

This review explores advanced materials for next-generation solar cells and light-emitting devices, focusing on solution-processable semiconductors and quantum dots. It highlights experimental and computational strategies for enhanced performance and novel applications.

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Area of Science:

Materials Science
Solid-State Physics
Photovoltaics
Optoelectronics

Background:

Traditional inorganic semiconductor devices face limitations in next-generation solar cells and light-emitting technologies.
Emerging materials offer potential for improved performance and novel device architectures.
Both experimental synthesis and computational modeling are crucial for advancing these fields.

Purpose of the Study:

To review potent directions in designing advanced materials for next-generation solar cells and light-emitting technologies.
To focus on recent conceptual advances addressing key challenges in the field.
To highlight the impact of these advances on applied literature.

Main Methods:

Experimental synthesis and characterization of novel materials.
Device fabrication and performance evaluation.
Computational modeling, including optical properties and aggregation effects.
Advanced theoretical methods beyond linear-response time-dependent density functional theory.

Main Results:

Exploration of solution-processable materials for easier fabrication.
Design strategies for dopant-free charge transport materials.
Advances in two-dimensional conjugated polymeric semiconductors.
Development of colloidal quantum dot assemblies for optoelectronic applications.
Insights into correlation effects and thermally activated fluorescence modeling.

Conclusions:

Significant progress is being made in designing advanced materials for solar cells and light-emitting devices.
Solution processability and dopant-free designs are key for future technologies.
Quantum dots and 2D polymers show great promise.
Advanced computational methods are essential for understanding and predicting material properties.