Analytical methods for organosulfate detection in aerosol particles: Current status and future perspectives

Organosulfates (OSs) are well-known water-soluble constituents of atmospheric aerosol particles. They are formed from multiphase reactions between volatile organic compounds (VOCs) and their photooxidation products, and acidic sulfate originating from biogenic and anthropogenic sources in the atmosphere. Although the analytical procedures used to measure OSs, including sampling, pre-treatment, and instrumental detection, have advanced substantially in the last decade, there is still a need for accurate and standardized analysis procedures for the identification, quantification, and comparison of OSs in different regions. Additionally, there has no study focused on the health effects of OSs. This review outlines the analytical methods developed for OS detection during the last decade, highlighting both improvements and drawbacks. It also considers the future development of analytical methods for OS detection, and proposes the establishment of OSs screening method from the perspective of health effects to solve the problem of unknown health related OSs identification.