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Energy Dispersive X-ray Tomography for 3D Elemental Mapping of Individual Nanoparticles
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Three-dimensional nanothermometry below the diffraction limit.

J Thiem, S Spelthann, J Neumann

    Optics Letters
    |July 15, 2021
    PubMed
    Summary
    This summary is machine-generated.

    Lanthanide-doped nanothermometers offer sensitive temperature measurements. This study numerically optimized their spatial resolution using stimulated emission depletion microscopy, achieving sub-diffraction limit contactless temperature sensing.

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    Area of Science:

    • Nanotechnology
    • Optical microscopy
    • Materials science

    Background:

    • Lanthanide-doped nanothermometers provide sensitive temperature measurements (few %/K).
    • Their spatial resolution, crucial for applications, remains understudied and unoptimized.

    Purpose of the Study:

    • To numerically investigate and enhance the spatial resolution of nanothermometers.
    • To establish relationships between spatial and temperature resolution using advanced microscopy techniques.

    Main Methods:

    • Numerical simulations of nanothermometers.
    • Application of stimulated emission depletion (STED) microscopy principles.
    • Systematic variation of excitation and depletion beam parameters.

    Main Results:

    • Identified fundamental relationships between spatial and temperature resolution.
    • Predicted contactless temperature measurement below the diffraction limit.
    • Achieved a temperature resolution of ±1.25 K.
    • Analyzed the impact of sample thickness and position on resolution.

    Conclusions:

    • STED microscopy significantly improves nanothermometer spatial resolution.
    • Sub-diffraction limit contactless thermometry is feasible.
    • Potential for three-dimensional temperature mapping demonstrated.