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Updated: Oct 28, 2025

Combining Microfluidics and Microrheology to Determine Rheological Properties of Soft Matter during Repeated Phase Transitions
Published on: April 19, 2018
Microscopic interactions and emerging elasticity in model soft particulate gels
Minaspi Bantawa1, Wayan A Fontaine-Seiler1, Peter D Olmsted1
1Department of Physics, Institute for Soft Matter Synthesis and Metrology, Georgetown University, 37th and O Streets, N.W., Washington, D.C. 20057, United States of America.
Abstract:
We discuss a class of models for particulate gels in which the particle contacts are described by an effective interaction combining a two-body attraction and a three-body angular repulsion. Using molecular dynamics, we show how varying the model parameters allows us to sample, for a given gelation protocol, a variety of gel morphologies. For a specific set of the model parameters, we identify the local elastic structures that get interlocked in the gel network. Using the analytical expression of their elastic energy from the microscopic interactions, we can estimate their contribution to the emergent elasticity of the gel and gain new insight into its origin.

