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Area of Science:

  • Materials Science
  • Electrochemistry
  • Energy Storage

Background:

  • All-solid-state batteries (ASSBs) are a promising next-generation energy storage technology.
  • Sulfide-based solid electrolytes (SEs) exhibit high ionic conductivity, making them attractive for ASSBs.
  • Current sulfide-based ASSB technology faces challenges in air stability, electrode fabrication, and interfacial resistance.

Purpose of the Study:

  • To review recent developments addressing challenges in sulfide-based ASSBs.
  • To highlight advancements in materials, processing, and cell assembly for practical applications.
  • To encourage further research and development in sulfide-based ASSB technology.

Main Methods:

  • Enhancing air stability of sulfide SEs using the hard-soft acid-base (HSAB) theory.
  • Developing novel electrode fabrication techniques, including wet chemical coating and dry film processes.
  • Optimizing cell assembly and operation through the application of external pressure.

Main Results:

  • Strengthening metal-sulfur bonds improved air stability, though energy density and anode interface stability require further resolution.
  • Wet chemical coating processes adapted from lithium-ion batteries show promise, with solutions found for solvent-electrolyte-binder polarity mismatches.
  • Dry film processing offers potential for cost reduction and increased volumetric energy density.
  • External pressure application is crucial for improving interface stability and interparticle contacts, leading to high cell performance.

Conclusions:

  • Significant progress has been made in addressing key challenges for sulfide-based ASSBs.
  • Further research is needed to resolve remaining issues related to energy density and anode interface stability.
  • Continued expertise engagement from the battery community is vital for advancing practical sulfide-based ASSB technology.