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Updated: Oct 23, 2025

Sputter Growth and Characterization of Metamagnetic B2-ordered FeRh Epilayers
Published on: October 5, 2013
Subpicosecond metamagnetic phase transition in FeRh driven by non-equilibrium electron dynamics
Federico Pressacco1,2, Davide Sangalli3,4, Vojtěch Uhlíř5,6
1The Hamburg Centre for Ultrafast Imaging, Hamburg University, Hamburg, Germany. federico.pressacco@desy.de.
Ultrafast laser pulses can switch materials between magnetic states. This study reveals how light triggers a ferromagnetic phase in iron-rhodium (FeRh) within 350 femtoseconds via electronic band structure changes.
Area of Science:
- Condensed matter physics
- Ultrafast phenomena
- Magnetism
Background:
- Femtosecond light can induce phase transitions, tuning material properties on ultrafast timescales.
- First-order phase transitions often involve complex non-equilibrium states, hindering precursor detection.
Purpose of the Study:
- To elucidate the subpicosecond processes behind photoinduced ferromagnetic order in iron-rhodium (FeRh).
- To understand the role of electronic band structure modification in ultrafast phase transitions.
Main Methods:
- Time-resolved photoelectron spectroscopy.
- Ab-initio electron dynamics calculations.
Main Results:
- Photoexcitation modifies the electronic band structure, not just state occupation.
- Ferromagnetic order in FeRh is established 350 ± 30 fs after laser excitation.
- Ab-initio calculations suggest Rh-to-Fe charge transfer initiates the transition.
Conclusions:
- Light-induced changes in electronic band structure drive ultrafast phase transitions.
- Charge transfer plays a key role in generating ferromagnetic order in FeRh.
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