Organic-Inorganic Hybrid Luminescent Hydrogel Glued by a Cationic Polymeric Binder

Luminescent hydrogels have shown great potential in many fields, such as lighting, display, imaging, and sensing, because of their unique optical properties, biocompatibility, and easy processing. Organic-inorganic hybrid self-assembly can not only enhance the hydrogels' mechanical strength, but also retain their self-healing ability. Herein, a luminescent supramolecular hydrogel is reported, which is formed via self-assembly of the negatively charged Laponite nanosheets and cationic lanthanide coordination polymer. The corresponding results reveal that the multiple binding interaction between Laponite and the polymeric binder is vital for improving the mechanical performance of the obtained luminescent supramolecular hydrogel.